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- W2183675922 abstract "Abstract The first catalytic asymmetric dearomatization of 3‐methyl‐2‐vinylindoles has been established by using quinone monoimides as suitable electrophiles in the presence of chiral phosphoric acid, which afforded chiral indole derivatives bearing a quaternary stereogenic center in a chemospecific and highly enantioselective fashion (up to 81% yield, >99% ee ). The success of this reaction was enabled by the reactivity switch of 3‐methyl‐2‐vinylindoles, which has not been reported before. This reaction also represents the first catalytic asymmetric arylative dearomatization of vinylindoles, which will help confront the challenges in catalytic asymmetric arylative dearomatization and dearomatization of vinylindoles. magnified image" @default.
- W2183675922 created "2016-06-24" @default.
- W2183675922 creator A5020884276 @default.
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- W2183675922 creator A5041300808 @default.
- W2183675922 creator A5086163138 @default.
- W2183675922 date "2015-12-04" @default.
- W2183675922 modified "2023-10-18" @default.
- W2183675922 title "Catalytic Enantioselective Arylative Dearomatization of 3-Methyl-2-vinylindoles Enabled by Reactivity Switch" @default.
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- W2183675922 doi "https://doi.org/10.1002/adsc.201500901" @default.
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