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- W2187188880 abstract "In this report we introduce two novel techniques, lasermuon spin spectroscopy (laser-µSR) where laser excitation follows muon arrival to excite muoniated molecules and laser pump-muon magnetic resonance probe where laser excitation precedes muon arrival to excite molecules reacting with muonium or muoniated free radicals. Both these techniques employ laser excitation to produce a transient while the chemical dynamics of which are probed using muon spin spectroscopy (µSR). By using a tunable laser system it will be possible to measure the electronic and vibrational excitations of a muoniated centre. This will provide an independent tool for radical and site assignments for muon implanted samples. This report presents the proof of principle experiments, using timeresolved Zero-Field µSR (ZF-µSR), to observe the change upon 532 nm laser excitation in the ZF asymmetry of the radical adduct produced by excitation of powdered rose bengal. For the first time these pump-probe experiments extend muonium chemistry to the realm of excited states. The results enable the detection of muoniated molecules by their spin evolution after laser excitation; opening new opportunities to study the chemical dynamics of muoniated intermediates in excited states." @default.
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- W2187188880 date "2006-01-01" @default.
- W2187188880 modified "2023-09-27" @default.
- W2187188880 title "Laying the foundation for a muon-laser spectroscopy" @default.
- W2187188880 hasPublicationYear "2006" @default.
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