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• W2187950657 abstract "The discovery of fullerenes encapsulated inside single-wall carbon nanotubes (SWCNTs) by Smith et al. [Nature 396, 323 (1998)], provides a compelling opportunity to study the nanotubes using fullerenes as local prob es. It is reviewed herein, how fullerenes and magnetic fullerenes such as N@C60 and C59N, and 13 C enriched fullerenes can be used to yield unprecedented insight into the nanotube electronic, vibrational, and optical properties and into the growth of SWCNTs. Encapsulated C60 fullerenes are transformed to inner tubes by high temperature annealing. The unique, low defect concentration and well shielded nature of inner tubes makes them ideal to study the effect of diameter dependent treatments such as opening and closing of the tubes. Electron-spin resonance studies on the encapsulated magnetic fullerenes indicates a metallic-like finite density of states for an ensembl e SWCNT sample, which contradicts the current view of SWCNTs as containing separate metallic and semiconducting nanotubes. The linear spin chains of the encapsulated magnetic fullerenes is suggested as a building element for quantum information processing. The possibility to grow inner tubes from encapsulated fullerenes allows the isotope selective enrichment of the inner tubes if the source fullerene is 13 C enriched. Nuclear magnetic resonance on such samples evidences the presence of a low energy spin-gap which is thought to open due to a Peierls transition." @default.
• W2187950657 created "2016-06-24" @default.
• W2187950657 creator A5085380868 @default.
• W2187950657 date "2007-01-01" @default.
• W2187950657 modified "2023-09-26" @default.
• W2187950657 title "RECENT ADVANCES IN THE ELECTRONIC AND VIBRATIONAL STUDIES OF CARBON NANOTUBES USING FULLERENES AS LOCAL PROBES" @default.
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