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- W2188810340 abstract "Abstract A series of Al- and Fe-MFI zeolites was synthesized using a hydrothermal treatment, and nano-sized MFI zeolites were obtained by an emulsion method. UV–vis spectra and ac -NH 3 -TPD profiles demonstrated that Fe atoms were incorporated into the frameworks of the MFI structures and that almost all of the Fe 3+ species were well dispersed without forming bulky iron oxide particles. The selective production of iso-butylene from acetone was examined using Al- and Fe-MFI zeolites with different crystal sizes. The nano-sized MFI zeolite exhibited a long catalyst lifetime compared with the macro-sized MFI zeolite. Although iso-butylene is normally an intermediate during acetone conversion over zeolite catalysts, the weak acidity of the Fe-MFI zeolite suppressed the completion of excessive reaction, leading to high selectivity for iso-butylene." @default.
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- W2188810340 date "2016-04-01" @default.
- W2188810340 modified "2023-09-25" @default.
- W2188810340 title "Size-controlled synthesis of MFI metallosilicate and their catalytic performance on acetone to olefins reaction" @default.
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- W2188810340 doi "https://doi.org/10.1016/j.micromeso.2015.10.043" @default.
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