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- W2192865664 abstract "A comparative study has been performed on Ni2P/SiO2 catalysts prepared by: (i) conventional temperature-programmed reduction (TPR) of calcined precursors following wet impregnation of the support, (ii) TPR of a sol–gel prepared NiO/SiO2 precursor impregnated with NH4H2PO4 and (iii) a solution-phase reaction in the presence of the SiO2 support using Ni(acac)2 and trioctylphosphine. Catalyst characterization shows that the Ni2P prepared by the solution-phase method has a uniform particle size (7.5 ± 0.8 nm) and H species can easily transfer from the nickel sites to the SiO2 support on this catalyst. These properties result in a high NaBH4 methanolysis to hydrogen activity. In contrast, the sol–gel prepared Ni2P/SiO2 has a relatively high catalytic activity for phenol hydrodeoxygenation due to a higher concentration of Niδ+ species that act as Lewis acid sites and metal sites, and a higher Ni2P crystallinity." @default.
- W2192865664 created "2016-06-24" @default.
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- W2192865664 date "2015-12-01" @default.
- W2192865664 modified "2023-10-18" @default.
- W2192865664 title "Effect of preparation method on Ni2P/SiO2 catalytic activity for NaBH4 methanolysis and phenol hydrodeoxygenation" @default.
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- W2192865664 doi "https://doi.org/10.1016/j.ijhydene.2015.09.145" @default.
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