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• W219784764 abstract "We have measured total and coincident (with outgoing charge-state analyzed projectiles) ionization and fragmentation spectra of C60 and C70 following collisions with Xe4+ and Kr4+ at v = 0.06 a.u. Intact positive fullerene ions in charge states up to five (C605+ and C705+) are produced with both projectiles and for Kr4++C70 collisions we even observe a small C706+ peak. The C60/70-2m3+ (m=1–7) intensity distributions are predominantly associated with the stabilization of three electrons on the projectile (s=3) and are significantly different for Xe4+- and Kr4+-projectiles. On the other hand, we find remarkable similarities in the C3+-C11+ multi-fragmentation pattern regardless of projectile species (mass) although they are associated with closer encounters in which the projectile is fully neutralized (s=4). Simple Monte Carlo calculations of nuclear and electronic loss processes show that both these contributions are very similar in glancing Xe4++C60 and Kr4++C60 collisions, suggesting that frontal (and more violent) collisions are strongly suppressed under the present experimental conditions. Nevertheless it is surprising that the more distant collisions (s=3) are projectile mass dependent, while the closer collisions (s=4) are not. This indicates that this simple approach (although it reproduces more advanced quantum mechanical calculations for slow collisions with singly charged atomic ions rather well) is not valid for a comprehensive description of the energy transfer processes in the present collision systems involving projectiles of higher charge states." @default.
• W219784764 created "2016-06-24" @default.
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• W219784764 date "2005-01-01" @default.
• W219784764 modified "2023-09-24" @default.
• W219784764 title "Electron transfer and fragmentation in fullerene collisions" @default.
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