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- W2201718945 abstract "Abstract The layered Ni-rich oxide LiNi 0.8 Co 0.1 Mn 0.1 O 2 cathode has been significantly attractive due to its large reversible capacity (∼200 mAh g −1 ). However, the inherent poor cycling stability of the Ni-based cathode materials is always a serious issue for restricting its commercialization. In this paper, we introduced Li 2 MnO 3 as an electrochemical inactive component in Ni-rich oxide LiNi 0.8 Co 0.1 Mn 0.1 O 2 to stabilize its structure. The modified LiNi 0.8 Co 0.1 Mn 0.1 O 2 composites with low-content Li 2 MnO 3 were prepared by a solid-state reaction process. The results from XRD structure refinement and SAED confirm that Li 2 MnO 3 phase exists homogeneously in the composites. The modified LiNi 0.8 Co 0.1 Mn 0.1 O 2 composites with inactive Li 2 MnO 3 show much better cycling stability and stable average discharge voltage compared with the pristine one when charged to 4.5 V. Especially, the modified LiNi 0.8 Co 0.1 Mn 0.1 O 2 composite with 10% Li 2 MnO 3 (LNCMO-1090) delivers a reversible capacity of 207 mAh g −1 and keeps 155 mAh g −1 after 100 cycles at 20 mA g −1 (0.1C), corresponding to a capacity retention of 75%, while LiNi 0.8 Co 0.1 Mn 0.1 O 2 could only maintain a capacity of 128 mAh g −1 with a capacity retention of 59% after 100 cycles. The improved cycling performance of the Li 2 MnO 3 -containing electrode could be attributed to the stabilized effect of Li 2 MnO 3 on the electrode surface structure, as evidenced by the lower charge-transfer resistance." @default.
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- W2201718945 date "2016-01-01" @default.
- W2201718945 modified "2023-10-01" @default.
- W2201718945 title "Improving the Cycling Performance of the Layered Ni-Rich Oxide Cathode by Introducing Low-Content Li 2 MnO 3" @default.
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- W2201718945 doi "https://doi.org/10.1016/j.electacta.2015.12.080" @default.
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