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• W2203502308 abstract "Abstract The overlithiation and delithiation behaviors of sol-gel formed LiNi 0.75 Co 0.25 O 2 are investigated in this work. As an insertion host material, LiNi 0.75 Co 0.25 O 2 is cycled in a broad working potential range of 1.35–4.3 V. It shows two lithiation platforms at 1.75/3.6 V and only one reverse delithiation platform at 3.7 V. The long lithiation platform at 1.75 V is attributed to the overlithiation behavior of LiNi 0.75 Co 0.25 O 2 . Although overlithiation reaction takes place below 2.0 V, LiNi 0.75 Co 0.25 O 2 can maintain electrochemical reversibility during the initial 20 cycles. To study the overlithiation/delithiation process, the structural evolution of LiNi 0.75 Co 0.25 O 2 is thoroughly observed by in-situ X-ray diffraction method. It can be found that the electrochemical reaction between LiNi 0.75 Co 0.25 O 2 and Li in 1.35–4.3 V is a reversible process, which is associated with a single-phase transition process above 3.0 V and a two-phase transformation below 2.0 V. This result not only demonstrates the high structural and electrochemical reversibility of LiNi 0.75 Co 0.25 O 2 in 1.35–4.3 V, but also proves the improved structural stability of LiNi 0.75 Co 0.25 O 2 via partial replacement of Ni by Co in layered LiNiO 2 ." @default.
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• W2203502308 date "2016-02-01" @default.
• W2203502308 modified "2023-09-25" @default.
• W2203502308 title "In-situ X-ray diffraction study on the structural reversibility of lithium nickel cobalt oxide in a broad electrochemical window of 1.35–4.3 V" @default.
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• W2203502308 doi "https://doi.org/10.1016/j.electacta.2015.12.200" @default.
• W2203502308 hasPublicationYear "2016" @default.
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