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• W2209593538 endingPage "497" @default.
• W2209593538 startingPage "443" @default.
• W2209593538 abstract "We explore the nature of glass-formation in variable spatial dimensionality ($d$) based on the generalized entropy theory, a synthesis of the Adam-Gibbs model with direct computation of the configurational entropy of polymer fluids using an established statistical mechanical model. We find that structural relaxation in the fluid state asymptotically becomes Arrhenius in the $drightarrowinfty$ limit and that the fluid transforms upon sufficient cooling above a critical dimension near $d=8$ into a dense amorphous state with a finite positive residual configurational entropy. Direct computations of the isothermal compressibility and thermal expansion coefficient, taken to be physical measures of packing frustration, demonstrate that these fluid properties strongly correlate with the fragility of glass-formation." @default.
• W2209593538 created "2016-06-24" @default.
• W2209593538 creator A5030026152 @default.
• W2209593538 creator A5044313983 @default.
• W2209593538 creator A5052757593 @default.
• W2209593538 date "2016-09-16" @default.
• W2209593538 modified "2023-09-23" @default.
• W2209593538 title "ENTROPY THEORY OF POLYMER GLASS-FORMATION IN VARIABLE SPATIAL DIMENSION" @default.
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