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- W2214671142 abstract "The Boson peak (BP) of deeply cooled confined water is studied by using inelastic neutron scattering (INS) in a large interval of the (P, T) phase plane. By taking into account the different behavior of such a collective vibrational mode in both strong and fragile glasses as well as in glass-forming materials, we were able to determine the Widom line that characterizes supercooled bulk water within the frame of the liquid-liquid phase transition (LLPT) hypothesis. The peak frequency and width of the BP correlated with the water polymorphism of the LLPT scenario, allowing us to distinguish the “low-density liquid” (LDL) and “high-density liquid” (HDL) phases in deeply cooled bulk water.Moreover, the BP properties afford a further confirmation of theWidom line temperature T W as the (P, T) locus in which the local structure of water transforms from a predominately LDL form to a predominately HDL form." @default.
- W2214671142 created "2016-06-24" @default.
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- W2214671142 date "2015-10-01" @default.
- W2214671142 modified "2023-10-12" @default.
- W2214671142 title "The Boson peak in confined water: An experimental investigation of the liquid-liquid phase transition hypothesis" @default.
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- W2214671142 doi "https://doi.org/10.1007/s11467-015-0487-8" @default.
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