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- W2216493408 abstract "Bimetallic Ni-Pd nanoparticles on two different acidic mesoporous silica supports, Al- SBA-15 and Al-TUD-1, were evaluated for the hydro-dehydroxylation cascade reaction of cyclohexanol to cyclohexane. The hydro-dehydroxylation (Fig. 1) is an interesting and important model reaction due to the presence of similar oxygen-based functional groups in biomass. To use biomass as an energy source however, such highly oxygenated materials have to be catalytically converted to alkanes (Cortright et al2002; Huber et al2006) A cascade reaction however necessitates the use of multifunctional catalysts where different active sites are needed for the separate steps in the cascade. In the case presented here, the acidic silica supports act as the catalyst for the dehydration of cyclohexanol, whereas the metal sites function as the catalyst for the hydrogenation of the cyclohexene. Another objective of this work is the capability of such catalysts to resist poisoning by sulfur compounds present in real biomass. One approach to overcome this problem is the usage of bimetallic nanoparticles where one metal is sacrificed for the benefit of the other (Azad et al 2007; Bartholomew 2001)." @default.
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- W2216493408 date "2011-01-01" @default.
- W2216493408 modified "2023-09-24" @default.
- W2216493408 title "Bimetallic Ni-Pd acidic catalysts for a hydro-dehydroxylation cascade reaction" @default.
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