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- W2216572023 abstract "We report on the large-scale synthesis of highly oriented ultrathin MoO3 layers using a simple and low-cost atmospheric pressure by van der Waals epitaxy growth on muscovite mica substrates. By this method we are able to synthetize high quality centimeter-scale MoO3 crystals with thicknesses ranging from 1.4 nm (two layers) up to a few nanometers. The crystals can be easily transferred to an arbitrary substrate (such as SiO2) by a deterministic transfer method and extensively characterized to demonstrate the high quality of the resulting crystal. We also study the electronic band structure of the material by density functional theory calculations. Interestingly, the calculations demonstrate that bulk MoO3 has a rather weak electronic interlayer interaction and thus it presents a monolayer-like band structure. Finally, we demonstrate the potential of this synthesis method for optoelectronic applications by fabricating large-area field-effect devices (10 micrometers by 110 micrometers in lateral dimensions), finding responsivities of 30 mA/W for a laser power density of 13 mW/cm2 in the UV region of the spectrum and also as an electron acceptor in a MoS2-based field-effect transistor." @default.
- W2216572023 created "2016-06-24" @default.
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- W2216572023 date "2016-05-27" @default.
- W2216572023 modified "2023-10-14" @default.
- W2216572023 title "Centimeter-Scale Synthesis of Ultrathin Layered MoO<sub>3</sub> by van der Waals Epitaxy" @default.
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- W2216572023 doi "https://doi.org/10.1021/acs.chemmater.6b01505" @default.
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