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• W2218743034 abstract "The oxidative behavior of aqueous sulfur dioxide has been assessed on a polycrystalline platinum electrode using cyclic voltammetry with variation in applied experimental parameters. Parameters varied include the acid concentration, reaction temperature, and lower potential limit . Three distinctly different oxidation scenarios were identified. These are defined by and, at , acid concentration as well. Observed oxidation scenarios include a limited response (scenario 1), catalytic oxidation (scenario 2), and reaction inhibition (scenario 3). Scenario 1 required an activation energy of with a Tafel slope of and transfer coefficient of . Scenario 2 was found to have a different reaction mechanism to scenario 1 , displaying faster reaction kinetics and catalytically improved oxidation onset . The onset of scenario 2 oxidation was dependent on oxidation kinetics, not thermodynamics, with . The variable response of the electrode is discussed in terms of sulfur species adsorption, including the reductive formation of adsorbed sulfur at potentials less than 0.5 V, and the adsorption of sulfur dioxide with varying adsorption strength." @default.
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• W2218743034 date "2010-01-01" @default.
• W2218743034 modified "2023-10-10" @default.
• W2218743034 title "The Electrochemical Oxidation of Aqueous Sulfur Dioxide" @default.
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• W2218743034 doi "https://doi.org/10.1149/1.3458860" @default.
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