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- W2219201102 abstract "In this work, we have used a Monte-Carlo simulation technique to study two-letter (AB) quasirandom copolymers with quenched primary structure, which were generated via surface-induced computer-aided sequence design, following a general concept first introduced by us for a solution of polymer globules [1–4] (for a recent review, see Ref. [26]). Two different approaches have been employed: (i) a “coloring” (i.e., chemical modification) of partially adsorbed homopolymer chains and (ii) a copolymerization near a surface. In the former case, AB copolymers were prepared by adsorbing a bare homopolymer chain onto a flat substrate, after which its adsorbed segments were converted to type A ones, and its unadsorbed segments to type B ones. The second approach represents an irreversible radical copolymerization of selectively adsorbed A and B monomers with different affinity to a surface. We have shown that the statistical properties of the copolymer sequences obtained in these two ways exhibit well-pronounced long-range correlations in distribution of different monomer units along the chain. In particular, the primary structure of copolymers generated via the “coloring” procedure is similar to that known for proteinlike copolymers [1–4,10]. On the other hand, the copolymers obtained from polymerizing monomers selectively adsorbed onto a flat substrate demonstrate a specific quasi-gradient primary structure under the preparation conditions studied in this work. In addition, some characteristics of the adsorbed single chains (statistics of trains, loops, and tails) have been also investigated." @default.
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- W2219201102 date "2004-01-01" @default.
- W2219201102 modified "2023-09-23" @default.
- W2219201102 title "Copolymers with Long-Range Correlations: Sequence Design Near a Surface" @default.
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- W2219201102 doi "https://doi.org/10.1007/1-4020-2340-5_6" @default.
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