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- W2220451863 abstract "Electrocatalysis is key to the efficient interconversion of elec. and chem. energies, an important component of future energytechnologies. We have developed new electrocatalysts for the oxygen redn. reaction (ORR), incorporating proton relays in thesecond coordination sphere. Iron-tetrakis(2-carboxyphenyl)porphyrin chloride is an active, stable, and unusually selective ORRelectrocatalyst in acidic acetonitrile, reducing O_2 almost entirely to H_2O rather than H_2O_2. The related tetrakis(2-pyridyl)porphyrin complex is also a relatively selective ORR electrocatalyst in acidic water, despite the long distance between thepyridyl nitrogen atoms and the iron center. The role of the proton relays, and now complexes with flexible tripodal ligands andpendent tertiary amines, will be discussed. New developments in the electrocatalysis of water oxidn. by copper-bipyridinespecies will also be presented." @default.
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- W2220451863 date "2013-04-01" @default.
- W2220451863 modified "2023-09-24" @default.
- W2220451863 title "New electrocatalysis for dioxygen reduction and water oxidation" @default.
- W2220451863 hasPublicationYear "2013" @default.
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