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- W2222148843 abstract "Abstract Highly selective catalysts for methanol synthesis from CO 2 and H 2 are required for increasing the process efficiency that actually produces large amounts of CO. The understanding of the Cu–ZnO synergy allowed the possibility to design core–shell catalysts of the type Cu@ZnO x with enhanced selectivity for methanol. This type of core–shell structure was synthesized with variable compositions and the catalytic efficiency as well as the physicochemical properties were scrutinized in order to build structure–reactivity relationships. Zn migration is responsible for the formation of the Cu x Zn (1− x ) O y active phase. The experimental results were compared with theoretical calculations based on a geometrical model taking into account the amount of Zn migrated. A direct correlation was found between theory and experiment. Finally, a linear correlation of catalyst activity versus Zn migrated is shown for three different catalyst designs, thus confirming that a high Zn migration is needed for obtaining an efficient methanol synthesis catalyst." @default.
- W2222148843 created "2016-06-24" @default.
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- W2222148843 date "2016-11-01" @default.
- W2222148843 modified "2023-10-10" @default.
- W2222148843 title "The Cu–ZnO synergy in methanol synthesis Part 3: Impact of the composition of a selective Cu@ZnO core–shell catalyst on methanol rate explained by experimental studies and a concentric spheres model" @default.
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- W2222148843 doi "https://doi.org/10.1016/j.jcat.2015.12.005" @default.
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