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- W2222159211 abstract "New compos~tiong radient solid electrolytes are developed which have application in high temperature solid state galvanic sensors and provide a new tool for thermodynamic measurements. The electrolyte consists oi a solid solution between two ionic conductors with a common mobile ion and spatial variation in composition of otber coxup nents. Incorporation of the composite electrolyte in sensors permits the use oi dissimilar gas electrodes. It is demonsuated, both experimentall y and theoretically, that the composition gradient of the relativeiy immobile species does not give rise to a diffusion potential.The emi of a cell is determined by the activity of the mobile species atthe two eiectrodes. The thermodynamic properties of solid solutions can be measured using the gradient solid electrolyte. The experimental stuay is based on model systems A?(COj)x(S04)l-x (A=Na,K),where S .aria across the electrolyte. The functionally gradient solid electrolytes used for activity measurements consist of pure carbonateat one ena and the solid solution under stuav at the other. The identical vaiues of activity, obtained h m t hree different modes of operation of the ceil. indicate unit transport number for the ddi metal ion in the graciient electrolyte. Tlle activities in the solid solutions exhibitmoderate positive deviations from Raoult 's law." @default.
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- W2222159211 date "1994-01-01" @default.
- W2222159211 modified "2023-09-24" @default.
- W2222159211 title "Application of composition gradient solid electrolytes in sensors and thermodynamic measurements" @default.
- W2222159211 hasPublicationYear "1994" @default.
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