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- W2226161745 abstract "The loss of internal pores, a process known as physical aging, inhibits the long-term use of the most promising gas-separation polymers. Previously we reported that a porous aromatic framework (PAF-1) could form a remarkable nanocomposite with gas-separation polymers to stop aging. However, PAF-1 synthesis is very onerous both from a reagent and reaction-condition perspective, making it difficult to scale-up. We now reveal a highly dispersible and scalable additive based on α,α'-dichloro-p-xylene (p-DCX), that inhibits aging more effectively, and crucially almost doubles gas-transport selectivity. These synergistic effects are related to the intimately mixed nanocomposite that is formed though the high dispersibility of p-DCX in the gas-separation polymer. This reduces particle-size effects and the internal free volume is almost unchanged over time. This study shows this inexpensive and scalable polymer additive delivers exceptional gas-transport performance and selectivity." @default.
- W2226161745 created "2016-06-24" @default.
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- W2226161745 date "2016-01-08" @default.
- W2226161745 modified "2023-09-30" @default.
- W2226161745 title "Hypercrosslinked Additives for Ageless Gas-Separation Membranes" @default.
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- W2226161745 doi "https://doi.org/10.1002/anie.201508070" @default.
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