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- W2226268833 abstract "The effective synthesis of two-dimensional transition metal dichalcogenides alloy is essential for successful application in electronic and optical devices based on a tunable band gap. Here we show a synthesis process for Mo1-xWxS2 alloy using sulfurization of super-cycle atomic layer deposition Mo1-xWxOy. Various spectroscopic and microscopic results indicate that the synthesized Mo1-xWxS2 alloys have complete mixing of Mo and W atoms and tunable band gap by systematically controlled composition and layer number. Based on this, we synthesize a vertically composition-controlled (VCC) Mo1-xWxS2 multilayer using five continuous super-cycles with different cycle ratios for each super-cycle. Angle-resolved X-ray photoemission spectroscopy, Raman and ultraviolet-visible spectrophotometer results reveal that a VCC Mo1-xWxS2 multilayer has different vertical composition and broadband light absorption with strong interlayer coupling within a VCC Mo1-xWxS2 multilayer. Further, we demonstrate that a VCC Mo1-xWxS2 multilayer photodetector generates three to four times greater photocurrent than MoS2- and WS2-based devices, owing to the broadband light absorption." @default.
- W2226268833 created "2016-06-24" @default.
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- W2226268833 date "2015-07-23" @default.
- W2226268833 modified "2023-10-14" @default.
- W2226268833 title "Controllable synthesis of molybdenum tungsten disulfide alloy for vertically composition-controlled multilayer" @default.
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- W2226268833 doi "https://doi.org/10.1038/ncomms8817" @default.
- W2226268833 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4525162" @default.
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