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- W2226595659 abstract "Abstract Although hydrocarbon production from unconventional reservoirs, the so-called shale gas, has exploded recently, reliable predictions of resource availability and extraction are missing because conventional tools fail to account for their ultra-low permeability and complexity. Here, we use molecular simulation and statistical mechanics to show that continuum description—Darcy’s law—fails to predict transport in shales nanoporous matrix (kerogen). The non-Darcy behaviour arises from strong adsorption in kerogen and the breakdown of hydrodynamics at the nanoscale, which contradict the assumption of viscous flow. Despite this complexity, all permeances collapse on a master curve with an unexpected dependence on alkane length. We rationalize this non-hydrodynamic behaviour using a molecular description capturing the scaling of permeance with alkane length and density. These results, which stress the need for a change of paradigm from classical descriptions to nanofluidic transport, have implications for shale gas but more generally for transport in nanoporous media." @default.
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- W2226595659 date "2015-04-22" @default.
- W2226595659 modified "2023-10-18" @default.
- W2226595659 title "Subcontinuum mass transport of condensed hydrocarbons in nanoporous media" @default.
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- W2226595659 doi "https://doi.org/10.1038/ncomms7949" @default.
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