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- W2227421798 abstract "There is very little information available about the dynamics of radical+radical interactions. These processes are important in combustion being chain termination steps as well as generating new molecular species. To study these processes, a new experimental apparatus has been constructed to investigate radical-radical dynamics. The first radical or atomic species is produced with a known concentration in a microwave discharge flow system. The second is produced by pulsed laser photolysis of a suitable photolyte. The time dependence of individual rovibrational states of the product is followed by absorption of a continuous infrared laser. This approach will allow the reaction of interest to be differentiated from other radical reactions occurring simultaneously. The experimental approach is highly versatile, being able to detect a number of molecular species of particular interest to combustion processes such as water, methane, acetylene etc. at the state specific level. State specific infrared absorption coefficients of radicals can be measured in situ allowing for the determination of the absolute concentrations and hence branching ratios for reactions having multiple reaction pathways." @default.
- W2227421798 created "2016-06-24" @default.
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- W2227421798 date "1998-03-06" @default.
- W2227421798 modified "2023-09-24" @default.
- W2227421798 title "Time-resolved infrared absorption studies of the dynamics of radical reactions." @default.
- W2227421798 hasPublicationYear "1998" @default.
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