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- W2227554983 abstract "A modified imidazole, namely guanidimidazole (GIm) was designed and synthesized as a novel quaternizing- and cross-linking agent for alkaline polymer electrolyte membrane fabrication. The resulting membrane was more alkali tolerant and swelling resistant than that quaternized purely by 1-methylimidazole owing to the enhanced resonance and cross-linking ability of GIm, the former confirmed by a LUMO (lowest unoccupied molecular orbital) energy calculation. The membrane also showed good ionic conductivity, mechanical strength and thermal stability. A H2/O2 fuel cell using the synthesized membrane showed a peak power density of 39 mW cm−2 at 50 °C. This work preliminarily demonstrates the beneficial effect of imidazole modification by both experimental and computational investigation; it provides a new cation design strategy that may potentially achieve simultaneous improvement of alkali stability and swelling resistance of alkaline electrolyte membranes." @default.
- W2227554983 created "2016-06-24" @default.
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- W2227554983 date "2016-03-01" @default.
- W2227554983 modified "2023-10-07" @default.
- W2227554983 title "Guanidimidazole-quanternized and cross-linked alkaline polymer electrolyte membrane for fuel cell application" @default.
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- W2227554983 doi "https://doi.org/10.1016/j.memsci.2015.12.012" @default.
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