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- W2227974312 abstract "Silver is an ideal candidate for surface plasmon resonance (SPR)-based applications because of its great optical cross-section in the visible region. However, the uses of Ag in plasmon-enhanced spectroscopies have been limited due to their interference via direct contact with analytes, the poor chemical stability, and the Ag+ release phenomenon. Herein, we report a facile chemical method to prepare shell-isolated Ag nanoparticle/tip. The as-prepared nanostructures exhibit an excellent chemical stability and plasmonic property in plasmon-enhanced spectroscopies for more than one year. It also features an alternative plasmon-mediated photocatalysis pathway by smartly blocking “hot” electrons. Astonishingly, the shell-isolated Ag nanoparticles (Ag SHINs), as “smart plasmonic dusts”, reveal a ∼1000-fold ensemble enhancement of rhodamine isothiocyanate (RITC) on a quartz substrate in surface-enhanced fluorescence. The presented “smart” Ag nanostructures offer a unique way for the promotion of ultrahigh sensitivity and reliability in plasmon-enhanced spectroscopies." @default.
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- W2227974312 date "2015-10-23" @default.
- W2227974312 modified "2023-10-03" @default.
- W2227974312 title "“Smart” Ag Nanostructures for Plasmon-Enhanced Spectroscopies" @default.
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- W2227974312 doi "https://doi.org/10.1021/jacs.5b09682" @default.
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