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- W2228582453 abstract "We report a comprehensive study on the interactions between cationic surfactant homologues CnTAB (n = 12, 14, and 16) with negatively charged cellulose nanocrystals (CNCs). By combining different techniques, such as isothermal titration calorimetry (ITC), surface tension, light scattering, electrophoretic mobility, and fluorescence anisotropy measurements, we identified two different driving forces for the formation of surface induced micellar aggregates. For the C12TAB surfactant, a surfactant monolayer with the alkyl chains exposed to the water is formed via electrostatic interactions at low concentration. At a higher surfactant concentration, micellar aggregates are formed at the CNC surface. For the C14TAB and C16TAB systems, micellar aggregates are formed at the CNC surface at a much lower surfactant concentration via electrostatic interactions, followed by hydrophobic interactions between the alkyl chains. At higher surfactant concentration, charge neutralization and association of the surfactant decorated CNC aggregates led to flocculation." @default.
- W2228582453 created "2016-06-24" @default.
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- W2228582453 date "2016-01-14" @default.
- W2228582453 modified "2023-10-14" @default.
- W2228582453 title "Structural and Energetic Studies on the Interaction of Cationic Surfactants and Cellulose Nanocrystals" @default.
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- W2228582453 doi "https://doi.org/10.1021/acs.langmuir.5b03893" @default.
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