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- W2231694781 abstract "A conceptual process is outlined for the conversion of natural gas to liquid transport fuels by the novel technique of catalytic oxidative coupling of methane. Methane coupling to higher hydrocarbons has been. conducted in 30 mm and 60 mm dia. fluidised-bed reactors, with methane conversions up to 40% being achieved at isothermal conditions using methane/oxygen mixtures without diluents. When operated at the same contact time the 30 mm and 60 mm reactors had similar performances. At 850 degreesC the selectivity to hydrocarbons decreased dramatically with increasing contact time. At lower temperatures the reduction in selectivity with increased contact time was less severe. Axial gas concentration profiles through the catalyst bed in the 60 mm reactor showed that at 850 C there was a rapid consumption of oxygen and formation of products in the bottom section of the reactor followed by a net loss of hydrocarbon in the oxygen-free zone of the catalyst bed. It is believed that this was due to carbon formation on the catalyst and this carbon was continuously circulated back to the oxygen-containing zone of the bed and combusted." @default.
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- W2231694781 date "1989-01-01" @default.
- W2231694781 modified "2023-09-28" @default.
- W2231694781 title "The oxidative coupling of methane to higher hydrocarbons - process concepts and reaction engineering aspects" @default.
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