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- W2233133225 abstract "Core–shell nanocomposites based on Au nanoparticle@zinc–iron-embedded porous carbons (Au@Zn–Fe–C) derived from metal–organic frameworks were prepared as bifunctional electrocatalysts for both oxygen reduction reaction (ORR) and hydrogen evolution reaction (HER). A single Au nanoparticle of 50–100 nm in diameter was encapsulated within a porous carbon shell embedded with Zn–Fe compounds. The resulting Au@Zn–Fe–C hybrids exhibited apparent catalytic activity for ORR in 0.1 M KOH (with an onset potential of +0.94 V vs RHE, excellent stability and methanol tolerance) and for HER as well, which was evidenced by a low onset potential of −0.08 V vs RHE and a stable current density of 10 mA cm–2 at only −0.123 V vs RHE in 0.5 M H2SO4. The encapsulated Au nanoparticles played an important role in determining the electrocatalytic activity for ORR and HER by promoting electron transfer to the zinc–iron-embedded porous carbon layer, and the electrocatalytic activity was found to vary with both the loading of the gold..." @default.
- W2233133225 created "2016-06-24" @default.
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- W2233133225 date "2016-01-12" @default.
- W2233133225 modified "2023-09-30" @default.
- W2233133225 title "Core–Shell Nanocomposites Based on Gold Nanoparticle@Zinc–Iron-Embedded Porous Carbons Derived from Metal–Organic Frameworks as Efficient Dual Catalysts for Oxygen Reduction and Hydrogen Evolution Reactions" @default.
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- W2233133225 doi "https://doi.org/10.1021/acscatal.5b02302" @default.
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