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- W2233819953 abstract "With the aim of developing a DNA sequencing methodology, we theoretically examine the feasibility of using nanoplasmonics to control the translocation of a DNA molecule through a solid-state nanopore and to read off sequence information using surface-enhanced Raman spectroscopy. Using molecular dynamics simulations, we show that high-intensity optical hot spots produced by a metallic nanostructure can arrest DNA translocation through a solid-state nanopore, thus providing a physical knob for controlling the DNA speed. Switching the plasmonic field on and off can displace the DNA molecule in discrete steps, sequentially exposing neighboring fragments of a DNA molecule to the pore as well as to the plasmonic hot spot. Surface-enhanced Raman scattering from the exposed DNA fragments contains information about their nucleotide composition, possibly allowing the identification of the nucleotide sequence of a DNA molecule transported through the hot spot. The principles of plasmonic nanopore sequencing can be extended to detection of DNA modifications and RNA characterization." @default.
- W2233819953 created "2016-06-24" @default.
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- W2233819953 date "2015-10-01" @default.
- W2233819953 modified "2023-10-17" @default.
- W2233819953 title "Plasmonic Nanopores for Trapping, Controlling Displacement, and Sequencing of DNA" @default.
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- W2233819953 doi "https://doi.org/10.1021/acsnano.5b04173" @default.
- W2233819953 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4660389" @default.
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