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• W2238006851 abstract "Augmenting fluorescence intensity is of vital importance to the development of chemical and biochemical sensing, imaging and miniature light sources. Here we report an unprecedented fluorescence enhancement with a novel architecture of multilayer three-dimensional colloidal photonic crystals self-assembled from polystyrene spheres. The new technique uses a double heterostructure, which comprises a top and a bottom layer with a periodicity overlapping the excitation wavelength (E) of the emitters, and a middle layer with a periodicity matching the fluorescence wavelength (F) and a thickness that supports constructive interference for the excitation wavelength. This E-F-E double heterostructure displays direction-dependent light trapping for both excitation and fluorescence, coupling the modes of photonic crystal with multiple-beam interference. The E-F-E double heterostructure renders an additional 5-fold enhancement to the extraordinary FL amplification of Rhodamine B in monolithic E CPhCs, and 4.3-fold acceleration of emission dynamics. Such a self-assembled double heterostructure CPhCs may find significant applications in illumination, laser, chemical/biochemical sensing, and solar energy harvesting. We further demonstrate the multi-functionality of the E-F-E double heterostructure CPhCs in Hg (II) sensing." @default.
• W2238006851 created "2016-06-24" @default.
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• W2238006851 date "2015-09-24" @default.
• W2238006851 modified "2023-10-10" @default.
• W2238006851 title "Anomalous Fluorescence Enhancement from Double Heterostructure 3D Colloidal Photonic Crystals–A Multifunctional Fluorescence-Based Sensor Platform" @default.
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• W2238006851 doi "https://doi.org/10.1038/srep14439" @default.
• W2238006851 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4585865" @default.
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