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• W2243384804 abstract "Transient optical anisotropy in the hexagonal manganite YMnO 3 excited by linearly and circularly polarized laser pulses has been observed. The photo-induced anisotropy was investigated by the pump-probe technique based on a femtosecond Ti:sapphire laser generating optical pulses at the photon energy of 1.55 eV. Temporal and spectral dependencies of the photo-induced optical rotation and ellipticity were analyzed by a theoretical model considering ultrafast population and relaxation processes near the interband transitions from the hybridized O 2− (2 p )-Mn 3+ (3 d ) (Γ 1 ) to the Mn 3+ (3d 3 z2−r2 ) (Γ 5 ) states at photon energies of the laser excitation. Very short relaxation time of ~10 fs, which is the Raman coherence time between the excited Γ 5 | x > and Γ 5 |y> states, has been determined. It is found that this coherence time is much shorter than a charge relaxation time of ~500 fs between the Γ 5 |x,y> and Γ 1 |g> states for the interband electronic transition Γ 1 →Γ 5 ." @default.
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• W2243384804 date "2015-07-01" @default.
• W2243384804 modified "2023-09-26" @default.
• W2243384804 title "Femtosecond Photo-Induced Phenomena in Multiferroic Hexagonal Manganite YMnO₃" @default.
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• W2243384804 doi "https://doi.org/10.4028/www.scientific.net/ssp.233-234.149" @default.
• W2243384804 hasPublicationYear "2015" @default.
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