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- W2247404884 abstract "We present a novel type of rod-coil graft copolymer containing a polyphenylene backbone linked with poly(ethylene oxide) (PEO) side chains. Such graft copolymers manifest unprecedented temperature-dependent one-dimensional (1D) and two-dimensional (2D) self-assembly in solution. At 20 °C, which is higher than the crystallization temperature (Tc) of the PEO chains, the achiral graft copolymers self-organize into nanoribbons that twist into ∼30 μm ultralong helices with controlled pitch depending on the grafting ratio of the PEO chains. At 10 °C, which is lower than the Tc, quadrangular multilayer sheets of over 10 μm in lateral size are obtained. To our knowledge, this work presents the first example of controlled self-assembly of graft polymers into 1D helix and 2D sheet superstructures." @default.
- W2247404884 created "2016-06-24" @default.
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- W2247404884 date "2015-09-04" @default.
- W2247404884 modified "2023-10-14" @default.
- W2247404884 title "Temperature-Dependent Multidimensional Self-Assembly of Polyphenylene-Based “Rod–Coil” Graft Polymers" @default.
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- W2247404884 doi "https://doi.org/10.1021/jacs.5b07487" @default.
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