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• W2252645531 startingPage "7096" @default.
• W2252645531 abstract "A proof of principle for the use of Diels–Alder chemistry as a thermoreversible cross-linking tool for rubber products is demonstrated. A commercial ethylene-propylene rubber grafted with maleic anhydride has been thermoreversibly cross-linked in two steps. The pending anhydride rings were first modified with furfurylamine to graft furan groups onto the rubber backbone. These pending furans were cross-linked with a bismaleimide via a Diels–Alder coupling reaction. The newly formed Diels–Alder cross-links break at elevated temperatures (>150 °C) and can be re-formed by thermal annealing (50–70 °C). Reversibility of the rubber network was proven with infrared spectroscopy and on the basis of the mechanical properties. Furthermore, reversibility was also shown in a practical way, i.e., by cutting the used material into pieces and pressing them into new samples displaying comparable mechanical properties (impossible for conventionally cross-linked rubbers). The physical properties of the resulting products are comparable to those of conventionally cross-linked EPDM rubber and superior compared to those of their non-cross-linked precursors." @default.
• W2252645531 created "2016-06-24" @default.
• W2252645531 creator A5013172607 @default.
• W2252645531 creator A5025676098 @default.
• W2252645531 creator A5084738855 @default.
• W2252645531 creator A5090097550 @default.
• W2252645531 date "2015-09-16" @default.
• W2252645531 modified "2023-10-16" @default.
• W2252645531 title "Use of Diels–Alder Chemistry for Thermoreversible Cross-Linking of Rubbers: The Next Step toward Recycling of Rubber Products?" @default.
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• W2252645531 doi "https://doi.org/10.1021/acs.macromol.5b01422" @default.
• W2252645531 hasPublicationYear "2015" @default.
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