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- W2252763528 abstract "A tale of two catalysts: One was the best α-arylation catalyst, one was the worst (it gave only γ-arylation). Their opposite regioselectivity in a unique umpolung C−H arylation of palladium azapentadienyl intermediates enabled the selective synthesis of allylic amine and enamine derivatives (see scheme). A cation–π interaction with the heterobimetallic Pd/Na NiXantphos catalyst is proposed to be responsible for the unusual γ-regioselectivity." @default.
- W2252763528 created "2016-06-24" @default.
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- W2252763528 date "2016-02-05" @default.
- W2252763528 modified "2023-09-23" @default.
- W2252763528 title "Palladium‐Catalyzed C−H Arylation of α,β‐Unsaturated Imines: Catalyst‐Controlled Synthesis of Enamine and Allylic Amine Derivatives" @default.
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- W2252763528 doi "https://doi.org/10.1002/anie.201509757" @default.
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