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• W2252872783 startingPage "876" @default.
• W2252872783 abstract "Hypervalent alkylsilicates represent new and readily accessible precursors for the generation of alkyl radicals under photoredox conditions. Alkyl radicals generated from such silicates serve as effective hydrogen atom abstractors from thiols, furnishing thiyl radicals. The reactive sulfur species generated in this manner can be funneled into a nickel-mediated cross-coupling cycle employing aromatic bromides to furnish thioethers. The serendipitous discovery of this reaction and its utilization for the thioetherification of various aryl and heteroaryl bromides with a diverse array of thiols is described. The S-H selective H atom abstraction event enables a wide range of functional groups, including those bearing protic moieties, to be tolerated." @default.
• W2252872783 created "2016-06-24" @default.
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• W2252872783 creator A5043162152 @default.
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• W2252872783 date "2016-02-08" @default.
• W2252872783 modified "2023-10-16" @default.
• W2252872783 title "Thioetherification via Photoredox/Nickel Dual Catalysis" @default.
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• W2252872783 doi "https://doi.org/10.1021/acs.orglett.6b00208" @default.
• W2252872783 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4854196" @default.
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