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• W2257320199 abstract "The quasi-one-dimensional conductor Li0.9Mo6O17 has been of great interest because of its unusual properties. It has a conducting phase with properties different from a simple Fermi liquid, a poorly understood insulating phase as indicated by a metal-insulator crossover (a mystery for over 30 years), and a superconducting phase which may involve spin triplet Cooper pairs as a three-dimensional (p-wave) non-conventional superconductor. Recent evidence suggests a density wave (DW) gapping regarding the metal-insulator crossover. However, the nature of the DW, such as whether it is due to the change in the charge state or spin state, and its relationship to the dimensional crossover and to the spin triplet superconductivity, remains elusive. Here by performing (7)Li-/(95)Mo-nuclear magnetic resonance (NMR) spectroscopy, we directly observed the charge state which shows no signature of change in the electric field gradient (nuclear quadrupolar frequency) or in the distribution of it, thus providing direct experimental evidences demonstrating that the long mysterious metal-insulator crossover is not due to the charge density wave (CDW) that was thought, and the nature of the DW gapping is not CDW. This discovery opens a parallel path to the study of the electron spin state and its possible connections to other unusual properties." @default.
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• W2257320199 date "2016-02-08" @default.
• W2257320199 modified "2023-10-06" @default.
• W2257320199 title "Direct observation of charge state in the quasi-one-dimensional conductor Li0.9Mo6O17" @default.
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• W2257320199 doi "https://doi.org/10.1038/srep20721" @default.
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