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- W2258858632 abstract "The electrochemical properties and phase stabilities of the multi-component olivine compound LiMn1/3Fe1/3Co1/3PO4 are studied experimentally and with first principles calculation. The formation of the solid solution between LiMnPO4, LiFePO4, and LiCoPO4 at this composition is confirmed by XRD patterns and the calculated first principles energy. The experimental and first principles results indicate that there are three distinct regions in the electrochemical profile at QOCPs of ca. 3.5 V, 4.1 V, and 4.7 V, which are attributed to Fe/Fe, Mn/Mn, and Co/Coredox couples, respectively. However, exceptionally large polarization is observed only for the region near 4.1 V of Mn3+/Mn2+ redox couples, implying the intrinsic charge transfer problem of Mn. An ex-situ XRD study reveals that the reversible onephase reaction of Li extraction/insertion mechanism prevails, unexpectedly, for all lithium compositions of LixMn1/3Fe1/3Co1/3PO4 (0 ≤ x ≤ 1) at room temperature. The well-ordered, non-nanocrystalline (less than 1% Li – M disorder and a few hundred nanometer size particle) olivine electrode is demonstrated to be operated solely in a onephase behavior (Figure 1)." @default.
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- W2258858632 date "2010-01-01" @default.
- W2258858632 modified "2023-09-27" @default.
- W2258858632 title "Study on Multi-Components Olivine Cathode: Combined First Principles Calculations and Experiments" @default.
- W2258858632 doi "https://doi.org/10.1149/ma2010-03/1/346" @default.
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