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- W2262912252 abstract "The iron complex [FeH(CO) (PNP)] (PNP = N(CH2CH2PiPr2)2) is a highly active catalyst for ammonia borane dehydrocoupling at room temperature. Mainly linear polyaminoborane is obtained upon release of 1 equiv of H2. Mechanistic studies suggest that both hydrogen release and B–N coupling are metal-catalyzed and proceed via free aminoborane. Catalyst deactivation results from reaction with free BH3 that is formed by aminoborane rearrangement. Importantly, borane trapping with a simple amine allows for the observation of a TON that is unprecedented for a well-defined base metal catalyst." @default.
- W2262912252 created "2016-06-24" @default.
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- W2262912252 date "2015-11-09" @default.
- W2262912252 modified "2023-10-16" @default.
- W2262912252 title "Highly Active Iron Catalyst for Ammonia Borane Dehydrocoupling at Room Temperature" @default.
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- W2262912252 doi "https://doi.org/10.1021/acscatal.5b02406" @default.
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