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• W2262954927 abstract "Abstract Valerate esters as a new class of cellulosic transportation fuels showed great industrial prospect. Here we developed a non-noble Ni/HZSM-5 bifunctional catalyst with excellent stability for the cascade transformation of levulinic acid to valerate esters. The acidity-regulation of Ni/HZSM-5 catalyst by potassium addition decreased the strong acidity, meanwhile tuned the proportion of Bronsted acidity/Lewis acidity. Coke analysis indicated that acidity-regulation by potassium addition changed the heavier coke component (alkylated poly-aromatics) to the lighter one (alkylated mono-aromatics), thus effectively prolonged the lifetime of Ni/HZSM-5 catalyst in fixed-bed reactor. The relationship of the nature of coke deposits and the acidity-regulation of catalysts could contribute to intensively understand the catalyst deactivation and the choice of stable catalyst for upgrading of biomass and its platform molecules." @default.
• W2262954927 created "2016-06-24" @default.
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• W2262954927 date "2016-07-01" @default.
• W2262954927 modified "2023-10-02" @default.
• W2262954927 title "Acidity-regulation for enhancing the stability of Ni/HZSM-5 catalyst for valeric biofuel production" @default.
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• W2262954927 doi "https://doi.org/10.1016/j.apcatb.2016.02.026" @default.
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