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- W2264509718 abstract "A significant amount of research is taking place to create energy storage concepts beyond the lithium ion battery and to utilize alternative ions, such as Na, Ca, or Mg, to name a few. This has been a challenge, as materials that work well to store lithium do not necessarily function for other ions. Crystalline germanium (Ge) represents such an example: Li can be readily inserted and extracted but not Na. However, by amorphizing the crystalline Ge nanowires with an initial lithiation step, Ge can be readily and reversibly sodiated. Here, we examine the sodiation and desodiation processes that occur in Ge nanowires using real-time in situ transmission electron microscopy (TEM). Amorphous germanium (a-Ge) nanowires exhibit a 300% expansion in volume upon sodiation, which corresponds approximately to Na1.6Ge, which indicates a higher than expected capacity to store Na, i.e., compared to NaGe. When the nanowires desodiate they form pores. The pores disappear when the nanowire is again sodiated. The nanowires ..." @default.
- W2264509718 created "2016-06-24" @default.
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- W2264509718 date "2016-02-10" @default.
- W2264509718 modified "2023-10-09" @default.
- W2264509718 title "Germanium as a Sodium Ion Battery Material: <i>In Situ</i> TEM Reveals Fast Sodiation Kinetics with High Capacity" @default.
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- W2264509718 doi "https://doi.org/10.1021/acs.chemmater.6b00200" @default.
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