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- W2268204620 abstract "The presence of Al atoms in tetrahedral and octahedral coordination in the crystal structure of ..gamma..-Al/sub 2/O/sub 3/ is responsible for the difference in potentials for these atoms close to the nucleus and, consequently, the difference in binding energy for the core electrons. In the x-ray photoelectron spectrum of ..gamma..-Al/sub 2/O/sub 3/, the line generated upon photoionization of the Al 2s shell has a complex shape (a maximum and a shoulder on the low-binding energy side). Its separation into two components show that their relative intensity reflects the ratio of Al atoms in the oxide having respectively the coordination numbers 4 and 6. The difference in binding energy for Al 2s for the two types of atoms is 0.7 eV, which agrees with data on calculation of the charge in oxide clusters. On the basis of the calculation results for the Al atoms by the Hartree-Fock-Dirac-Slater method, it is shown that the effective electronic configuration of the atoms may also exert an effect on the binding energy of the core electrons." @default.
- W2268204620 created "2016-06-24" @default.
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- W2268204620 date "1985-09-01" @default.
- W2268204620 modified "2023-09-27" @default.
- W2268204620 title "Coordination nonequivalence of aluminum atoms in. gamma. -Al/sub 2/O/sub 3/" @default.
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