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• W2272914043 abstract "In this study, sol–gel processing was proposed to prepare a creatinine (Cre)-imprinted molecularly imprinted polymer (MIP). The intermolecular interaction constituted by the cross-linkers, i.e., 2-acrylamido-2-methylpropane-sulfonic acid (AMPS) and aluminium ion (Al3+), was studied and compared in order to form a confined matrix that promises the effectiveness of molecular imprinting. In view of the shape recognition, the hydrogen bonded Cre-AMPS did not demonstrate good recognition of Cre, with Cre binding found only at 5.70 ± 0.15 mg g−1 of MIP. Whilst, MIP cross-linked using Al3+ was able to attain an excellent Cre adsorption capacity of 19.48 ± 0.64 mg g−1 of MIP via the stronger ionic interaction of Cre-Al3+. Based on the Scatchard analysis, a higher Cre concentration in testing solution required greater driving force to resolve the binding resistance of Cre molecules, so as to have a precise Cre binding with shape factor. The molecular recognition ability of Cre-MIP in present work was shape-specific for Cre as compared to its structural analogue, 2-pyrrolidinone (2-pyr), by an ideal selectivity coefficient of 6.57 ± 0.10. In overall, this study has come up with a practical approach on the preparation of MIP for the detection of renal dysfunction by point-of-care Cre testing." @default.
• W2272914043 created "2016-06-24" @default.
• W2272914043 creator A5016623056 @default.
• W2272914043 creator A5037911153 @default.
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• W2272914043 date "2016-04-01" @default.
• W2272914043 modified "2023-10-02" @default.
• W2272914043 title "Configuration control on the shape memory stiffness of molecularly imprinted polymer for specific uptake of creatinine" @default.
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• W2272914043 doi "https://doi.org/10.1016/j.apsusc.2016.02.076" @default.
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