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• W2274403732 abstract "Abstract Methyl formate (MF) is a valuable platform molecule, the industrial production of which is far from being green. In this contribution, TiO 2 ‐supported Pd( z )Pt(1− z ) catalysts were found to be effective in the green synthesis of methyl formate (MF)—at T =323 K and ambient pressure—through methanol (MeOH) oxidation. Two series of catalysts with similar bulk Pd/(Pd+Pt) molar ratios, z , were prepared; one by a water‐in‐oil microemulsion (MicE) method and the other by an incipient wetness impregnation (IWI). The MicE method led to more efficient catalysts owing to a weak influence of z on particle size distributions and nanoparticles composition. Pd( z )Pt(1− z )‐MicE catalysts exhibited strong synergistic effects for MF production but weak synergistic effects for MeOH conversion. The catalytic performance of Pd( z )Pt(1− z )‐MicE was superior to that of Pd( z )Pt(1− z )‐IWI catalysts despite the latter displaying synergetic effects during the reaction. The catalytic behavior of TiO 2 ‐supported Pd( z )Pt(1− z ) catalysts was explained from correlations between XRD, TEM, and X‐ray photoelectron spectroscopy characterizations." @default.
• W2274403732 created "2016-06-24" @default.
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• W2274403732 date "2016-02-17" @default.
• W2274403732 modified "2023-10-18" @default.
• W2274403732 title "Synergetic Behavior of TiO₂ -Supported Pd(<i>z</i> )Pt(1−<i>z</i> ) Catalysts in the Green Synthesis of Methyl Formate" @default.
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• W2274403732 doi "https://doi.org/10.1002/cctc.201501211" @default.
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