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• W2275014669 abstract "Studies of the catalyzed hydrogenation of carbon monoxide play a pivotal role in modern catalyst science. The reaction is exothermic whether it produces methane, methanol, high molecular weight hydrocarbons or alcohols. Thus, it makes fuels and chemicals from the synthetic gas feedstock, CO, and H2 that can be produced readily from methane or by the steam gasification of coal. By the early seventies, modern surface science reached such a level of maturity that its various techniques were employed for the CO hydrogenation studies. Low energy electron diffraction and electron microscopy were used to explore the catalyst surface structure, and electron spectroscopies (X-ray photoelectron, Auger and U.V. photoelectron-spectroscopies) were used to determine the surface composition and the oxidation states of surface atoms. Vibrational spectroscopies (high resolution electron energy loss and Fourier transform infrared) determined the structure of chemisorbed molecules, reaction intermediates, and molecular fragments. Solid state NMR and radioisotope labeling techniques were also employed extensively, and single crystal model catalysts explored the elementary reaction steps, the structure sensitivity of chemisorption, bond breaking, and bond formation. All these scientific investigations and the discovery of novel oxide supports, titanium oxide and zeolites permitted the development of new technologies that produce fuels or the desired chemicals with excellent selectivity. The transition metal or transition metal compound catalyst was used to control the elementary reaction, alkane, alkene or alcohol formation. The support oxide accelerated the metal catalyzed reaction steps or controlled the secondary reactions, the polymerization of the CHx fragments to produce linear or cyclic, aromatic products." @default.
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• W2275014669 date "1991-01-01" @default.
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• W2275014669 title "Chapter 11 The Catalyzed Hydrogenation of Carbon Monoxide: An Overview and Future Directions" @default.
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• W2275014669 doi "https://doi.org/10.1016/s0167-2991(08)60953-2" @default.
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