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- W2275603719 abstract "Band gap engineering of monolayer transition metal dichalcogenides, such as MoS2 and WS2, is essential for the applications of the two-dimensional (2D) crystals in electronic and optoelectronic devices. Although it is known that chemical mixture can evidently change the band gaps of alloyed Mo(1-x)W(x)S2 crystals, the successful growth of Mo(1-x)W(x)S2 monolayers with tunable Mo/W ratios has not been realized by conventional chemical vapor deposition. Herein, we developed a low-pressure chemical vapor deposition (LP-CVD) method to grow monolayer Mo(1-x)W(x)S2 (x = 0-1) 2D crystals with a wide range of Mo/W ratios. Raman spectroscopy and high-resolution transmission electron microscopy demonstrate the homogeneous mixture of Mo and W in the 2D alloys. Photoluminescence measurements show that the optical band gaps of the monolayer Mo(1-x)W(x)S2 crystals strongly depend on the Mo/W ratios and continuously tunable band gap can be achieved by controlling the W or Mo portion by the LP-CVD." @default.
- W2275603719 created "2016-06-24" @default.
- W2275603719 creator A5010215768 @default.
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- W2275603719 date "2016-02-22" @default.
- W2275603719 modified "2023-10-14" @default.
- W2275603719 title "Chemical Vapor Deposition of Monolayer Mo1−xWxS2 Crystals with Tunable Band Gaps" @default.
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- W2275603719 doi "https://doi.org/10.1038/srep21536" @default.
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