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- W2276064504 abstract "Despite residing in an energetically and structurally disordered landscape, the spin degree of freedom remains a robust quantity in organic semiconductor materials due to the weak coupling of spin and orbital states. This enforces spin-selectivity in recombination processes which plays a crucial role in optoelectronic devices, for example, in the spin-dependent recombination of weakly bound electron-hole pairs, or charge-transfer states, which form in a photovoltaic blend. Here, we implement a detection scheme to probe the spin-selective recombination of these states through changes in their dielectric polarizability under magnetic resonance. Using this technique, we access a regime in which the usual mixing of spin-singlet and spin-triplet states due to hyperfine fields is suppressed by microwave driving. We present a quantitative model for this behaviour which allows us to estimate the spin-dependent recombination rate, and draw parallels with the Majorana-Brossel resonances observed in atomic physics experiments." @default.
- W2276064504 created "2016-06-24" @default.
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- W2276064504 date "2015-10-06" @default.
- W2276064504 modified "2023-10-13" @default.
- W2276064504 title "Spin-dependent recombination probed through the dielectric polarizability" @default.
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- W2276064504 doi "https://doi.org/10.1038/ncomms9534" @default.
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