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• W2276907118 abstract "Conventional photocells suffer a fundamental efficiency threshold imposed by the principle of detailed balance, reflecting the fact that good absorbers must necessarily also be fast emitters. This limitation can be overcome by `parking' the energy of an absorbed photon in a dark state which neither absorbs nor emits light. Here we argue that suitable dark states occur naturally as a consequence of the dipole-dipole interaction between two proximal optical dipoles for a wide range of realistic molecular dimers. We develop an intuitive model of a photocell comprising two light-absorbing molecules coupled to an idealised reaction centre, showing asymmetric dimers are capable of providing a significant enhancement of light-to-current conversion under ambient conditions. We conclude by describing a roadmap for identifying suitable molecular dimers for demonstrating this effect by screening a very large set of possible candidate molecules." @default.
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• W2276907118 date "2016-11-10" @default.
• W2276907118 modified "2023-09-29" @default.
• W2276907118 title "Photocell Optimization Using Dark State Protection" @default.
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• W2276907118 doi "https://doi.org/10.1103/physrevlett.117.203603" @default.
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