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- W2277005702 abstract "Abstract The catalytic-oxidative evolution of the redox/spin states of a Fe-phthalocyanine (Fe-Pc) catalyst was studied by electron paramagnetic resonance spectroscopy. Under oxidative catalytic conditions, Fe-Pc may evolve via multiple redox/spin conformations. Axial ligation of imidazole, O 2 or t -Bu-OOH as oxidant, results in a complex multipath redox/spin landscape that was determined in detail herein. The high-spin conformations of Fe-Pc/imidazole evolve more slowly than the low-spin conformations. Catalytically active vs. inactive conformations were distinguished. A unified physicochemical catalytic reaction mechanism is discussed herein based on the distinct role of the various structural, spin and redox forms." @default.
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- W2277005702 date "2016-04-01" @default.
- W2277005702 modified "2023-10-17" @default.
- W2277005702 title "Oxidative catalytic evolution of redox- and spin-states of a Fe-phthalocyanine studied by EPR" @default.
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- W2277005702 doi "https://doi.org/10.1016/j.cplett.2016.02.032" @default.
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