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• W2277170771 abstract "Simultaneous control of the kinetics and thermodynamics of two different types of covalent chemistry allows pathway selectivity in the formation of hydrogelating molecules from a complex reaction network. This can lead to a range of hydrogel materials with vastly different properties, starting from a set of simple starting compounds and reaction conditions. Chemical reaction between a trialdehyde and the tuberculosis drug isoniazid can form one, two, or three hydrazone connectivity products, meaning kinetic gelation pathways can be addressed. Simultaneously, thermodynamics control the formation of either a keto or an enol tautomer of the products, again resulting in vastly different materials. Overall, this shows that careful navigation of a reaction landscape using both kinetic and thermodynamic selectivity can be used to control material selection from a complex reaction network." @default.
• W2277170771 created "2016-06-24" @default.
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• W2277170771 date "2015-11-10" @default.
• W2277170771 modified "2023-10-11" @default.
• W2277170771 title "Gelation Landscape Engineering Using a Multi-Reaction Supramolecular Hydrogelator System" @default.
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• W2277170771 doi "https://doi.org/10.1021/jacs.5b06988" @default.
• W2277170771 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4655419" @default.
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