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• W2277595754 abstract "The localization and distribution of the Mn2+ ions in two sol–gel deposited ZnO films doped with different manganese concentrations were investigated by electron paramagnetic resonance spectroscopy and analytical transmission electron microscopy. In the lightly doped sample the Mn2+ ions are mainly localized substitutionally at isolated tetrahedrally coordinated Zn2+ sites in both crystalline ZnO nanograins (34%) and surrounding disordered ZnO (52%). In the highly doped ZnO film, a much smaller proportion of manganese substitutes Zn2+ in the crystalline and disordered ZnO (10%). The main amount (85%) of manganese aggregates in a secondary phase as an insular-like distribution between the ZnO nanograins. The remaining Mn2+ ions (14% and 5% at low and high doping levels, respectively) are localized at isolated, six-fold coordinated sites, very likely in the disordered intergrain region. Annealing at 600 °C induced changes in the Mn2+ ions distribution, reflecting the increase of the ZnO crystallization degree, better observed in the lightly doped sample." @default.
• W2277595754 created "2016-06-24" @default.
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• W2277595754 date "2017-02-01" @default.
• W2277595754 modified "2023-10-15" @default.
• W2277595754 title "Mn2+ ions distribution in doped sol–gel deposited ZnO films" @default.
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• W2277595754 doi "https://doi.org/10.1016/j.apsusc.2016.02.167" @default.
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