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• W2277660943 abstract "Abstract It is vitally important for opto-electronic organic devices to optimize the photo-excitation efficiency. One strategy would be the arrangement of molecules in the vicinity of metal nano-particles (MNPs) and the enhancement of photon absorption or emission due to the coupling of molecular transitions to MNP plasmon excitations. If two or more MNPs are placed in the proximity of a single molecule it would couple to the hybrid plasmon levels of the MNPs. The energetic position of these levels is directly related to the MNP arrangement and, thus, can be easily adopted to the molecular transitions. Using a density matrix methodology we investigate molecular excitation dynamics upon photon absorption in a dye molecule placed in the vicinity of spherical MNPs. Firstly, a system of two identical MNPs is considered and an absorption enhancement of three orders of magnitude is demonstrated. Secondly, a system of four identical MNPs symmetrically placed around the dye molecule is investigated. The different plasmon hybrid levels originated by different arrangements of MNPs make it possible to choose a large variety of molecules to be excited with high efficiency. This would be of particular interest for future applications." @default.
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• W2277660943 date "2016-05-01" @default.
• W2277660943 modified "2023-09-22" @default.
• W2277660943 title "Theory of plasmon enhanced molecular absorption: Effects of plasmon hybridization due to multiple metal nano-particle arrangement" @default.
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• W2277660943 doi "https://doi.org/10.1016/j.orgel.2016.02.015" @default.
• W2277660943 hasPublicationYear "2016" @default.
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