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- W2277974417 endingPage "2026" @default.
- W2277974417 startingPage "2019" @default.
- W2277974417 abstract "Chiral phosphoric acid-catalyzed enantioselective aza-Friedel–Crafts reaction of trifluoromethyl benzoxazinones with pyrroles is reported. Under mild conditions, a range of enantioenriched dihydrobenzoxazinones bearing trifluoromethylated quaternary stereocenters could be obtained in good to excellent yield and ee. A remarkable fluorine effect is observed, and preliminary mechanistic studies combined with theory calculations suggest that triple-hydrogen-bonding interactions hold the transition structure rigidly and allow the bulky substituents of the catalyst to influence the enantioselectivity." @default.
- W2277974417 created "2016-06-24" @default.
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- W2277974417 date "2016-02-22" @default.
- W2277974417 modified "2023-10-14" @default.
- W2277974417 title "Organocatalytic Asymmetric Synthesis of Dihydrobenzoxazinones Bearing Trifluoromethylated Quaternary Stereocenters" @default.
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- W2277974417 doi "https://doi.org/10.1021/acs.joc.5b02848" @default.
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